By Andrei A Kulikovsky
In gasoline cellphone research, the hole among primary electrochemical tactics and the engineering of gasoline telephone platforms is bridged by means of the actual modelling of gasoline cells. This quite new self-discipline goals to appreciate the elemental shipping and kinetic phenomena in a true phone and stack setting, paving the best way for more desirable layout and function. The author brings his new angle to the analytical modeling of gas cells to this crucial reference for power technologists. Covers contemporary advances and analytical options to quite a number difficulties confronted by way of strength technologists, from catalyst layer functionality to thermal balance presents designated graphs, charts and different instruments (glossary, index) to maximise R&D output whereas minimizing bills and time spent on dead-end researchPresents Kulikovsky's signature process (and the information to help it)-which makes use of "simplified" versions in response to idealized platforms, easy geometries, and minimum assumptions-enabling qualitative figuring out of the factors and results of phenomena
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Extra info for Analytical Modelling of Fuel Cells
Participants in electrochemical reactions are charged particles (positive and negative) and neutral molecules in the gaseous or liquid form. Any catalyst layer is thus a composition of three ingredients: electronic and ionic conductors and voids for gas/liquid supply. The reaction itself occurs on a surface of precious metal particles (typically Pt), which must be connected to the avenues for charged and neutral species transport. Functional models of such a complex structure are based on the idea of macrohomogeneous approach.
The considerable thickness of the active layer facilitates electrochemical conversion under these conditions. In the anode-supported SOFC, the anode thickness is about 1 mm (1000 µm) to provide mechanical stability of the cell sandwich. 6. In PEFCs the cathode side makes the largest contribution to voltage loss. This explains the great interest in CCL performance in these cells. We begin the analysis of CL performance with the cathode catalyst layer of a low-temperature hydrogen fuel cell. However, it should be emphasized that the performance of other catalyst layers of the cells considered in this book can be described by similar equations.
In combination with high power density (about 1 W cm−2 ), this makes SOFCs a very attractive power source for residential applications. 11). 11). The transport of O2− ions occurs in a ceramic electrolyte, typically yttria-stabilized zirconia (YSZ), which has sufficient ionic conductivity at temperatures above 600 ◦ C. At temperatures of 600-900 ◦ C the conversion of hydrocarbons (methane) to hydrogen can be organized in situ so that no special reforming equipment is necessary. This conversion is a purely chemical process, which does not involve charged particles.